Chemistry and Physics of Solar Cells

General

Main concept Solar cells

3 Charge collection

1 Light absorption

Why solar cells

Immense amount of solar energy reaches earth

Efficiency's has gone up and prices gone down

Sustainable method for creating energy

2 Charge seperation

Performance quantities

Jsc

FF

Voc

Structure

Elemental semiconductors = group IV elements

Group III+V elements can be used together

Quantum mechanics

Efficiency

Volume density (atoms/volume)

Surface density (atoms/area)

Introduction to quantum mechanics

Goal

Emerging PV (application)

Operations of solar cells (theory)

AM = Air mass = 1/cos(theta)

AM1.5 is the normal spectrum (1000W/m2)

High refractive index leads to reflection

Silicium has the diamond structure

GaAs has the zincblende structure

Polycrystallinity should be avoided --> intrabandgap states

Photovoltaic effect (work function) --> de broglie wavelength (L = h/p) --> Time dependent SE --> Time independent SE --> general solution free electron --> BC (infinite) well --> solution (infinite) well --> solution step potential --> Reflection/Transmission/Tunneling --> Formation energy bands

Quantum theory of solids

Semiconductor material

Equilibrium

No forces acting on the semiconductor

Intrinsic SC

Effective mass m*

Density of states

Kronig-penny 1d model

Formation energy bands in crystalline solids

Negative for holes = have opposite direction

The effective mass of electrons and holes takes into account the particle weight and all internal forces acting on it. F = m*a

m = h*2/d2E/dk2

Sharp energy bands = low effective mass

Broad energy bands = large effective mass

Fermi-dirac distribution function

Can be used to determine he probability that a state with energy E is filled.

Differential density of quantum states

For SC

Number of states per unit energy and volume

Vb

Cb

Depends on hole mass and Ev - E

Depends on electron mass and E-Ec

By assuming periodic step wise periodic potentials around atoms

Can be used to describe the energy state in solids with the bloch function phi = u(x)exp(ikx)

Resulting function: p'sin(aa)/aa + cos(aa) = cos(ka)

a = atom distance, alpha = measure for energy(root(2me/h2), p'= (barrier height (v0), barrier depth b, mass particle)

for certain energys the function on the left side is greater than |1|, cos(ka) can be maximal be |1| so for those energys there is no k- value/wavenumber--> origin band gap.

Bandgap energy can be determined by filling in the two alpha values at the same k-value

Amount of charge carriers

Pure SC with no impurities or lattice deffects

Extrinsic/doped SC

Addition of donor/acceptor atoms = doping

Dopant ionisation statistics

Electrons in CB

Holes in VB

Fermi position

Using density of states * fermi-dirac(simplif)

n0 = ni = Nc*exp(Ef-Ec)/kt

p0 = ni = Nv*exp(Ev-Ef)/kt

Nc = effective DOS

Dependent on electron mass/hole mass ratio

Types

n-type doping

p-type doping

The addition of group 5 element that have an extra electron that is loosely bound. Thermal excitation can excite these electron to the conduction band and a positive charge stays on the element

The addition of group 3 elements result in that it can take up an extra electron. Thermal excitation can excite electrons from the vb to the energy state above the vb that creates holes in the vb

Overcompensated SC

Temperature dependence

nd = Nd-Nd+

Nd = density of dopants

Nd+ = density of ionized dopant

nd = density of nonionized dopants

nd/(n0+nd)

Usually very small above 200 K

Vast energy levels above pull out all electrons

Semiconductor that contains both acceptor and donor atoms

Electrons are now the dominant charge carriers. n = ne

ni2 = p0*n0 still holds

Region 2 = Extrinsic >> intrinsic so T independent

Region 3(high T) = intrinsic >= extrinsic so no longer T ind (fermi back)

Region 1 = higher conductivity with T due to ionisation (100 k)

n-type overcompensated

p-type overcompensated

It behaves like intrinsic if both are present in same conc --> annihilation and ni2=n0*p0

2 1/8volume shell/Vk

Energies

Volume

Three dimensional potential well --> E = h2k2(x,y,z)/2m

Vk = (pi/a)^3

Fill in to get DOS

Integrate to get number of state between E and E + iets

ni2 = p0n0 = NvNc*exp(-Eg/kt)

So smaller bandgap = more cc

Both nv and nc are T dependent

Use to have constant sigma or to create junction

Dominant charge carriers are p0

Increases the fermi level

Decreases the fermi level

Relation fermi level/ conc

p0 = ni*exp(Efi-Ef)/kt

n0 = ni*exp(Ef-Efi)/kt

Use electroneutrality formula to determine final concentrations

Transport phenomena

Non-equilibrium
Excess charge carriers

Charge carrier Diffusion

Charge carrier drift

Flux = electron/hole drift + electron/hole diffusion

Due to an electric field

Due to an concentration gradient

J = e(munN+mupP)E + eDndn/dx - eDp*dp/dx

Drift current density

Inbalance in +k and -k = net momentum

J = Nevc = NemuE = e(munN+mup*P)E

Mobility

Increases with lower m* and longer scattertime

Factor causing scattering

Phonon scattering, mu = T^-1.5

Ionized inpurity scattering, mu = T^3/2/Ni

Goes with T^3/2 because electrons get less stuck

Hence electrons have higher mobility

Diffusion current density

J = eDndn/dx

Current follows direction of the holes

D = kbt*Mu/e

IPCE = photon to current efficiency

Generation and recombination

Ambipolar transport

Shine light/change T

Terminology

Generation = the creation of holes/electrons

Recombination = The annihilation of electron/holes

Equilibrium

Gn0=Gp0=Rn0=Rp0

Generation holes/electrons equal --> come in pairs

n = total conc = constant + dn(t)

no = thermal equilibrium electrons = constant

dn = excess electrons = n-n0

tau-n0 = excess minority carrier lifetime

gn' = excess generation rate

Rn' = excess recombination rate

Non-equilibrium

Minority carriers determine the properties

n*p = ni^2 does not hold anymore

Recombination kinetics

Radiative recombination

R = arn(t)p(t) (2nd order)

Low level injection = generation of charge carriers is small compared to the majority carriers. So p0>>dn or n0>>dp

Extrinsic SC + low-level injection

n-type, d(dp)/dt = -arn0*(dp(t)) = p(t)/tau-po

So majority carrier is a constant (+-first order)

Recombination lifetime

tau-no = 1/arPo

tau-po = 1/arN0

Continuity equation

Diffusion

Generation

Drift

Recombination

Movement of electrons and holes is coupled because an electric field will arise if they are seperated or have different diffusivities = Ambipolar diffussion

Can be made for both holes and electrons

Ambipolar transport equation

Depends only on the minority carrier

D' and mu' = ambipolar diffusion coeficient and mobility

Are functions of concentrations

But for extrinsic, low level injection. The diffusion coeficients are that of the minority carriers. So use faster minority = use p-type

Because majority carrier has much higher conductivity and can easily adjust

Simplification help solve the problem

Quasi fermi levels

Fermi levels of holes (Efp) and electrons (Efn) with excess carriers

Fermi level of majority carrier will not deviate much from Ef

Use the given that you can relate states using only the energy difference

p-type, d(dn)/dt= -ar(dn(t))*p0 = n(t)/tau-no

Trap assisted/ Non-radiative

Origin

Defects/Dangling bond in lattice or at the surface(diffusion gradient)

Non-bonding orbitals might give energy states inside the bandgap --> deep traps willl assist recombination

Usually faster than Radiative recombination

Processes

Electron from trap to CB

Hole from VB to trap

Electron from CB to trap

Hole from Trap to VB

Extrinsic semiconductor

N-type

P-type

Fermi level is above trap energy --> filled trap states

First recombination with excess holes (minority), then majority carrier will instantaniously follow

Fermi level is below trap energy --> empty trap states

First recombination with excess electrons (minority), then majority carrier will follow instantaniously

Low level injection, Et near Ef, Rp = CpNtdp = dp/tp0

Low level injection, Rn = CnNtdn = dn/tn0

Semiconductor device

PN-junction

Basic structure

Zero-applied bias

Reverse applied bias

Electric field

Space-charge width

Energy band diagram

Junction capacitance

One sided junction

Space charge width

Space charge region

Junction between an uniformly doped n-type and p-type material

Built-in potential barrier

Gauss law

Poisson equation

Region near juntion where complete depletion occurs

No carriers are present and drift/diffusion are in equilibrium

Because of diffusion of majority carriers

N-type side becomes positively charged

P-type side becomes negatively charged

dE = p/eta

-d^2(phi)/dx^2 = p/eta

Flat junctions

Constant E if uniformely doped

E = sigma/2eta

In equilibrium band bending must occur such that the fermi level (with conc term) of the n-type and p-type material are at the same level = no current

P-type increases in energy and n-type decreases (electrostatic)

Difference in energy Efp, Efn

Vbi = Efn-Efp = kT/e * ln(NaNd/ni^2)

Vbi is between 0 and the band gap energy

Vbi is difficult to go the bandgap = much doping required

Maximum energy that can be extracted

Electric field

Approx

Uniform

Fully depleted/ionized

Abrupt junction

p-region

n-region

Emax = -eNaxp/eta

Ndxn = Naxp

Always below zero

E = -e(Na)(xp-x)/eta

Potential in n-type region contains built in potentail vbi

Can be used to calculate space charge width = use formula

Depends on doping densities, Vbi and dielectric constant

W = xp + xn

|Emax| = 2 Vbi / W

Increases when applying a potential

Potential is applied such that n-type gets more positive and p-type gets more negative

Replace Vbi with Vbi+Vr in all formulas

Because doping remains the same

Charge that is extra stored when the SCR is increased

C' = eta/W

Can be determined via an (1/C^2) vs iets plot

When the doping densities differ so much that the space charge region is almost at one side. So if Na>>>Nd or Nd>>>Na

Forward applied bias

Potential barrier is lowered with e(Vbi-Va), such that diffusion can now overcome the potential. Electron flow from n to p and hole flow from p to n.

Nomenclature

Nn

N = electrons or holes n/p

n = in n-type or p-type = n,p,n0,p0

From forward bias to ideal diode current

Concentration profile minority carrier

Diffusive current

Non-idealities

Forward bias recombination current

Reverse bias generation current

Overal diode relation

Concentration mc next to SCR

Increases exponentially with Va

np=np0*exp(eva/kt)

Assumptions

Decreases exp with distance (rec)

g'=0

ss

E = 0 in neutral region

Quasi fermi level splitting is constant in SCR

If assumed no recombination in junction

Current = hole diffusive current + electron diffusive current

Ideal diode equation

Determined using ambipolar transport equation

E- field neutral region

Gradient of concentration profile next to SCR (xn,-xp)

J = Js * (exp(eva/kt)-1)

Js = reverse bias saturation current density

If Va < 0, -Js is maximum reached

To balance current away from SCR, there is a small gradient in majority carrier --> small electric field

Balance diode current with drift current majority carrier to obtain E

Small because majority carriers has much higher conductivity

Jgen = eniW/2t0

In SCR with n=p=0 there must be generation (via traps)

Derive R

So additional charges must be injected to compensate for recombination

Jrec = Jr0*exp(eVa/2kt)

Injected charges may recombine in SCR

Dominates at low applied potentials

J = Jd + Jrec = Js(exp(eVa/nkt)-1)

n = ideality factor between 1-2, 1 at high v, 2 at low v

The SCR decreases for an forward bias until the built in potential is reduced to zero = Voc

Quandrants pn junction diode

2nd

3th

1st

4th

Forward bias, consumes energy = LED

No current

Reverse bias, negative current, Photo diode

Forward bias, negative current, pv quadrant

Open potential < Vbi (entropic terms)

Metal-semiconductor junction

Semiconductor heterojunction

Metal SC ohmic contact

Schottsky barrier diode

General

When

At high V, the chance of recombination is much higher

Metal contacts are needed for charge extraction

Properties

Ideal juction

Non-ideal junction

Current-voltage relationship

Schottsky barrier loading

Interface states

When

Ef,p-type < Ef, metal

Metal gets into contact with semiconductor

Ef, n-type < Ef, metal

Ef, p-type > Ef, metal

Barrier that forms that prevent the diffusion of holes/electrons into the semiconductor in ss

Space charge region is completely in the semiconductor (no charges in metal = one sided juntion)

Nomenclature

X

Work function

From fermi-level metal to vacuum

From vacuum level to CB

Phim

Phis

Electron affinity

Ef, n-type > Ef, metal

For n-type there is a flow of electrons towards the metal

Schottsky barier

Phib0 = (Ec-Ef,m)/e = phim - X

Built-in potential

Vbi = Phib0 - (Ec -Ef,s)/e = Phib0 - phin

So difference CB to metal en CB in neutral SC

Difference fermi level metal and energy CB to metal

Vacuum level goes up in the SC

Remains the same, independent of applied bias

Is functioin of applied bias

Width SCR SC

Same as for an one sided juntion

The experimental Phibn can differ from the theoretical Phib0

Polarisation can occur that lowers the energy of electrons close to the metal --> barrier gets lower energy

Surface gets-charge due to traps at the surface

For many trap states: Charge occurs until Ef, surface = phim = phi0

Phi0 = local neutrality level of interface defects

Barrier height is now phi0-Xs ipv Phim - Xs

Flux depends on direction electrons, velocity, energy states, fermi dirac

J = Js(exp(eVa/kt)

The flux of electrons that have enough energy (Ec') to move to the metal

Js = A T^2*exp(-eVa/kt)

A = Richardson constant for thermionic emission

Barrier is now (Ec-Ef)

Favourable to have no resistance from electrons/holes flowing when positive voltage is applied

Solar cells

Thin films

Perovskite + Organic

1st generation(Si)

High efficiency Concepts + QDs

More rec = lower Voc

Watch out, use constants with cm

Behave via the rules of ohms law

General

Formula's get more complex because have not the same properties

Types

2 Bandgap partially in each other (energy allignment)

3 Bandgaps have no overlap (rare)

1 Bandgap inside the other (no charge T)

Junction between two different SC materials

Band diagram

Naming

Nn

n-n juntion are also now possible

Larger bandgap is denoted with capital letter

Fermi levels still equal

Because potential is the same at the interface, dEc and dEv must be unchanged at interface

Bending is now not that predictable

If fermi-level > Ec, highly doped at that position

Fabrication silicon

Production solar cell

Solar cell efficiency

Properties absorber layer

Light absorption

Charge separation

Charge extraction

Absorption Si low = indirect bandgap, need phonons

Should absorb 80-90% light

Using tricks (reflection)

Increasing layer size (300 um)

Generation rate g' = alpha*Iv(x)/hv

Number of electrons/hole pairs at position x s-1

During illumination, E-field pn junction will extract electrons to n-type and holes to p=type

Diffusive current at junction counteracts this = unfavourable

Long diffusion distances

lifetime

High mobilities

use electron minority

Better at low doping

Reduce trap states

Current I = IL - IS(exp(eV/nkt-1)

IL = light induced current

Unwanted diffusive current

Limiting cases

R = 0, J=Jsc=IL Short circuit current

R = inf J = 0

Occurs at Voc

Voc = nkT/e ln(1+IL/IS)

Voc increaes with light intensity

Voc decreases by recombination

Conversion efficiency = ImVm/Pin = JscVoc*FF/Pin

Fill factor = ImVm/IscVoc

Solar cell has power point tracking to extract as much power as possible. Power point can change depending on conditions (varies the external resistance)

Crystallinity silicon

Process

Series resistance should be as low as possilbe and shunt as high as possible --> can be optimized using fingers and bushbars

Obtaining pure silicon

Step 1 SiO2 + C --> Si + CO2 (metullurgical grade silicon)

Step 2 Si + 3HCl --> SiHCl3 + H2 --> Si + 3HCl (electronic grade)

99.999% purity required to have low trap states

Obtaining crystalline silicon

Czochralski process (Specific cooling to 1 crystal)

Float zone crystallisation (heated into 1 crystal)

Single (10 cm)

Multi (most used)

Poly (to much defects)

Higher crystallinity is more expensive but results in less grain boundaries

Screen printed solar cells

Put block in phosphor environment (800K) to n-dope outside (no abrupt juntion)

Cut away bottom n-type and screen print Al back contact

Start with silicon block (low doped p-type naturally)

Al diffuses into p-type --> heavely doped p+ --> pp+ junction that extracts holes

Than apply AR coating otherwise 30% reflection

Add silver contacts on top such that series resistance is low, shunt high

Good efficiency but more costly production method

Cheap but lower efficiency

Amorphous silicon

Polycrystalline

CI(G)S

Properties

Fermi levels are equal

Fermi levels not equal anymore

Thinner layers, less material needed

More defects, lower diffusion length

Stronger absorption (direct bandgap)

Cheaper production method

Properties

CdTe

'Efficient and cheap'

Economics

Cost per Wp (AM1.5)

BOS

Cost/m2

Lifetime

Grid parity

Cost per kWh

3 um thick

Absorption is stronger --> disordered state relaxes the dk=0 selection rule. In between (in)direct bandgap.

1 um thick

Doping of a-Si

Transport in a-Si

Fabrication of a-Si

Challanges

Diffusion

Drift

Way shorter diffusion length than thickness (low mob/lifetime)

Around same diffusion lengths as thickness

Many defects (dangling bond) 10^16 --> passivate with H (10^15)

Really hard because defect density is so high --> no effect

More efficient in a-Si (1 um)

Much shorter than thickness

Ld = muEtau

p-i-n juntion

Undoped i has very large SCR --> needed for drift extraction

To thick i = dead regions without E

Deposit Si using CVD

Use transparant conducting oxide as contact

Copper, indium, gallium, selenide

Toxicity of Cd

Price of Te

Defects at suface and grain boundaries

II-VI semiconductor with bandgap close to SQ limit

Has high defect density, treat with CdCl2 to go to 22% efficiency

Less toxic and has good bangap tunability

Perovskite solar cell

Organic solar cells

SC properties

Cell designs

Structure and composition

Tandem cells

Metal halide PRK

ABX3

B = metal (pb2+,Sn)

X = halide (I,Br,Cl)

A = cation (MA,Cs,FA)

Used for solar cell applications

Compostion influences bandgap

Cation

Halide

Metal

Eg, Cs>MA>FA

Eg, Cl>Br>I

Eg, Pb>Sn

Crystal structure

Orthorombic for T<161K (a niet b niet c)

Tetragonal for T>161K (at room T, a = b niet c)

Cubic for T>330 k

Strong absorption

Doping

Point defects

Results in self-doping

Occurs due to low bond strength

Can either be n or p-type defects

Structure PRK not suited for doping

Can change Ef, by altering precursor ratio

n-i-p configuration

p-i-n configuration

Transport layers should have large bandgaps and allign with the VB and CB

Four terminal tandem cell (seperate)

Two terminal tandem cell (needs current matching)

Fermi level splitting denotes Voc

Present developments

Configuration

Charge extraction

SC properties

Have low electron permitivity --> large exciton binding energy compared to kt--> exciton remains until charge separation

Can form VB and CB due to bonding of MOs

Molecules are held by VDW interactions and can easily be modified

Few charge carriers due to large bandgap and non-charged imperfections

Excition diffusives towards junction that seperates electron from hole using E-field

Diffusion length is very small --> need many interfaces inside material

TCO

Bulk heterojunction

Metal contact

Mixture of polymer and electron acceptor

Both have 3d structure to move hole/electron to contact with electronic hopping

Efficiencies over 10% and is cheap,flexible and easy to process

Optimize energy levels to reduce energy losses

Enhance charge transport

Reduce bandgap close to 1000 nm

Limitations of conversion

Quantum dots

Thermodynamic maximum efficiency

Methods to break SQ

Solid angle

Limit = Carnot efficiency = 1 - Tcold/Thot

Emitting and absorption of solar cell (use J=sigmaT^4)

Maximum ideal solar cell

1 sun

Maximum concentrated

Thermalisation (goes to CB +3KT^, in 10^-12s)

Fermi level splitting (thermo)

Absorbed efficiency

Maximum power point (FF)

SQ only assumes radiative recombination +AM1.5

Proven

Concentrator cells

Tandem and multijunction solar cells

Difficulties

Advantages

Difficulties

Advantages

More theoretical

Intermediate band solar cells

Upconversion

Downconversion

Concept solar cells

Carrier multiplication

SC behaviour

Colloidal SC nanocrystals

Bandgap

Difficulties

Part of sunlight seen by earth = A/r^2 (steradian)

This can be increases using a lense up to max 46200 times

Solar cell cannot use energy that it emmits

= etacar times etaemm

67% (with tandem)

86%

Absorb hole spectrum, no thermilisation

Absorb more light

More energy use of absorbed light

Expensive

Lattice matching

Current matching (monolithic)

Max = 44% for two junctions

No contacts in between

Lowest current limits whole cell

Depends on light spectrum

Use alloying to steer lattice size

Otherwise many dangling bonds

Uses tunnel junctions

High dopant conc --> small SCR --> tunneling possible for electrons to recombine with holes in next layer

Higher efficiency

Less area solar cell needed

Voc increases (high IL)

FF increases = 1 - KT/Voc

Efficiency drops with temperature

High current means large voltage drop

Create energy band with electrons in the middle such that low energy photons are absorbed. But also lead to more recombination

2 small energy photons are combined to 1 photon

Can happen in some organic molecules and can be applied on the back of a solar cell.

To high photon energies are converted to two lower energy

Apply on surface SC but problems that created phons go up and down.

Depends on size crystals

Can be related to particle in the box = discrete energy levels

Enp = Eg + quantum confinement term + coulombic term

Tandem solar cell

Due to discrete energy levels, phonon creation is decreases, less thermilisation

Using different size PbS quantum dots

Hot carriers

Not yet made into solar cell

Energy of thermilisation of two created charge carriers excites electron to CB

Stronger effect in smaller QD

Quantum dots have large surface area and thus problems with surface recombination

Extract hot carriers in quantum dots by using extration far above CB