Spin dynamics in 2D materials

Objectives

Understand the time scaling of diffusion, explore the correlation between material dimension with such power law in time

Control the spin diffusion in the 2D material with such Hamiltonian engineering

Figure out the necessary decoupling to retrieve the coherent spin diffusion

Methods

Factors

Models

System composition : 2D crystal of spins

System dimension

Hamiltonian engineering

Spin diffusion measurement

Memory enhanced correlation protocol

Hartman-Hahn to polarize the system spins with NV center

Magnetization decay of nuclear spins probed with NV center

Monoisotopic hBN

13C enriched graphene

11B : spin 3/2 (quad. moment)

Nitrogen spins ?

Spin 1/2

2D: Monolayer

3D: Bulk

Intermediary: Bi/Tri-layer

Classical diffusion

1D exponent: 1/2

2D exponent: 1

3D exponent 3/2